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Quantum implementation of the unitary coupled cluster for simulating molecular electronic structure

Quantum implementation of the unitary coupled cluster for simulating molecular electronic structure

In classical computational chemistry, the coupled-cluster ansatz is one of the most commonly used $ab~initio$ methods, which is critically limited by its non-unitary nature. The unitary modification as an ideal solution to the problem is, however, extremely inefficient in classical conventional computation. Here, we provide the first experimental evidence that …