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Exploring the equivalence of causality-based and quantum mechanics-based sum rules for harmonic generation in nonlinear optical materials
The Kramers-Kronig relations and various oscillator strength sum rules represent strong constraints on the physical response of materials. In this work, taking inspiration from the well-established equivalence between $f-$sum rules and Thomas--Reiche--Kuhn sum rules in linear optics, we explore the connection between causality-based and quantum-mechanics-based sum rules in the context …