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First- and second-order magneto-optical effects and intrinsically anomalous transport in the two-dimensional van der Waals layered magnets <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mi>Cr</mml:mi><mml:mrow><mml:mi>X</mml:mi><mml:mi>Y</mml:mi></mml:mrow></mml:mrow><mml:mo> </mml:mo><mml:mrow><mml:mo>(</mml:mo><mml:mi>X</mml:mi><mml:mo>=</mml:mo><mml:mi mathvariant="normal">S</mml:mi><mml:mo>,</mml:mo><mml:mi>Se</mml:mi><mml:mo>,</mml:mo><mml:mi>Te</mml:mi><mml:mo>;</…
Recently, the two-dimensional magnetic semiconductor CrSBr has attracted considerable attention due to its excellent air-stable property and high magnetic critical temperature. Here, we systematically investigate the electronic structure, magnetocrystalline anisotropy energy, first-order magneto-optical effects (Kerr and Faraday effects), and second-order magneto-optical effects (Sch\"afer-Hubert and Voigt effects) as well as intrinsically …