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Manifestations of metastable criticality in the long-range structure of model water glasses

Manifestations of metastable criticality in the long-range structure of model water glasses

Much attention has been devoted to water's metastable phase behavior, including polyamorphism (multiple amorphous solid phases), and the hypothesized liquid-liquid transition and associated critical point. However, the possible relationship between these phenomena remains incompletely understood. Using molecular dynamics simulations of the realistic TIP4P/2005 model, we found a striking signature of …