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Radiation- and phonon-bottleneck--induced tunneling in the Fe <sub>8</sub> single-molecule magnet
We measure magnetization changes in a single crystal of the single-molecule magnet Fe8 when exposed to intense, short (⩽20 μs) pulses of microwave radiation resonant with the m = 10 to 9 transition. We find that radiation induces a phonon bottleneck in the system with a time scale of ∼5 …