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Ultrafast Control of Material Optical Properties via the Infrared Resonant Raman Effect

Ultrafast Control of Material Optical Properties via the Infrared Resonant Raman Effect

The Raman effect, inelastic scattering of light by lattice vibrations (phonons), produces an optical response closely tied to a material's crystal structure. Here we show that resonant optical excitation of IR and Raman phonons gives rise to a Raman-scattering effect that can induce giant shifts to the refractive index and …