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Low-dimensional quantum magnetism in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mi>Cu</mml:mi><mml:msub><mml:mrow><mml:mo>(</mml:mo><mml:mi>NCS</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:math> : A molecular framework material
Low-dimensional magnetic materials with spin-$\frac{1}{2}$ moments can host a range of exotic magnetic phenomena due to the intrinsic importance of quantum fluctuations to their behavior. Here, we report the structure, magnetic structure, and magnetic properties of copper ii thiocyanate, ${\mathrm{Cu}(\mathrm{NCS})}_{2}$, a one-dimensional coordination polymer which displays low-dimensional quantum magnetism. Magnetic …