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Low-temperature enhancement of ferromagnetic Kitaev correlations in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mi>α</mml:mi><mml:mo>−</mml:mo><mml:mi>Ru</mml:mi><mml:msub><mml:mi>Cl</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:mrow></mml:math>

Low-temperature enhancement of ferromagnetic Kitaev correlations in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mi>α</mml:mi><mml:mo>−</mml:mo><mml:mi>Ru</mml:mi><mml:msub><mml:mi>Cl</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:mrow></mml:math>

Kitaev-type interactions between neighbouring magnetic moments emerge in the honeycomb material ${\alpha}$-RuCl3. It is debated however whether these Kitaev interactions are ferromagnetic or antiferromagnetic. With electron energy loss spectroscopy (EELS) we study the lowest excitation across the Mott-Hubbard gap, which involves a d4 triplet in the final state and therefore …