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Wannier-function description of the electronic polarization and infrared absorption of high-pressure hydrogen

Wannier-function description of the electronic polarization and infrared absorption of high-pressure hydrogen

We have constructed maximally localized Wannier functions for prototype structures of solid molecular hydrogen under pressure, starting from local-density approximation and tight-binding Bloch wave functions. Each occupied Wannier function can be associated with two paired protons, defining a ``Wannier molecule.'' The sum of the dipole moments of these ``molecules'' always …