Precise Control of Molecular Dynamics with a Femtosecond Frequency Comb
Precise Control of Molecular Dynamics with a Femtosecond Frequency Comb
We present a general and highly efficient scheme for performing narrow-band Raman transitions between molecular vibrational levels using a coherent train of weak pump-dump pairs of shaped ultrashort pulses. The use of weak pulses permits an analytic description within the framework of coherent control in the perturbative regime, while coherent …