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Exotic (anti)ferromagnetism in single crystals of<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mtext>Pr</mml:mtext></mml:mrow><mml:mn>6</mml:mn></mml:msub><mml:msub><mml:mrow><mml:mtext>Ni</mml:mtext></mml:mrow><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mrow><mml:mtext>Si</mml:mtext></mml:mrow><mml:mn>3</mml:mn></mml:msub></mml:mrow></mml:math>
The ternary intermetallic compound, ${\text{Pr}}_{6}{\text{Ni}}_{2}{\text{Si}}_{3}$, is a member of a structure series of compounds based on a triangular structure where the number of Pr atoms in the prism cross section can be systematically varied. ${\text{Pr}}_{6}{\text{Ni}}_{2}{\text{Si}}_{3}$ contains two distinct Pr lattice sites which result in complex interactions between the magnetic ions. …