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Spin-Driven Ferroelectricity in Triangular Lattice Antiferromagnets<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mi>A</mml:mi><mml:msub><mml:mi>CrO</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math>(<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mi>A</mml:mi><mml:mo>=</mml:mo><mml:mi>Cu</mml:mi></mml:math>, Ag, Li, or Na)

Spin-Driven Ferroelectricity in Triangular Lattice Antiferromagnets<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mi>A</mml:mi><mml:msub><mml:mi>CrO</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math>(<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mi>A</mml:mi><mml:mo>=</mml:mo><mml:mi>Cu</mml:mi></mml:math>, Ag, Li, or Na)

The correlation between the dielectric and magnetic properties is investigated on the triangular-lattice antiferromagnets ACrO2 (A=Cu, Ag, Li, or Na) with a 120-degree spiral structure. For the A=Cu and Ag compounds with a delafossite structure, the ferroelectric polarization emerges with a spiral-spin order, implying strong coupling between ferroelectricity and the …