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Theory of excitonic second-harmonic generation in monolayer<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mi mathvariant="normal">MoS</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math>

Theory of excitonic second-harmonic generation in monolayer<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mi mathvariant="normal">MoS</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math>

Recent experimental results have demonstrated the ability of monolayer ${\mathrm{MoS}}_{2}$ to efficiently generate second harmonic fields with susceptibilities between 0.1 and 100 nm/V. However, few theoretical calculations exist with which to interpret these findings. In particular, it is of interest to theoretically estimate the modulus of the second harmonic response …