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Interplay of thermal and quantum spin fluctuations in the kagome lattice compound herbertsmithite

Interplay of thermal and quantum spin fluctuations in the kagome lattice compound herbertsmithite

We present a Raman spectroscopic investigation of the Herbertsmithite ZnCu3(OH)6Cl2, the first realization of a Heisenberg s=1/2 antiferromagnet on a perfect kagome lattice. The magnetic excitation spectrum of this compound is dominated by two components, a high temperature quasi elastic signal and a low temperature, broad maximum. The latter has …