Vacuum space charge effect in laser-based solid-state photoemission spectroscopy

Type: Article

Publication Date: 2010-01-01

Citations: 44

DOI: https://doi.org/10.1063/1.3273487

Abstract

We report a systematic measurement of the space charge effect observed in the few-picosecond laser pulse regime in laser-based solid-state photoemission spectroscopy experiments. The broadening and the shift of a gold Fermi edge as a function of spot size, laser power, and emission angle are characterized for pulse lengths of 6 ps and 6 eV photon energy. The results are used as a benchmark for an N-body numerical simulation and are compared to different regimes used in photoemission spectroscopy. These results provide an important reference for the design of time- and angle-resolved photoemission spectroscopy setups and next-generation light sources.

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  • Journal of Applied Physics - View
  • eScholarship (California Digital Library) - View - PDF
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